New paper: Gaussians for Electronic and Rovibrational Quantum Dynamics

Published as part of the Journal of Physical Chemistry A Virtual Special Issue “Attosecond Chemistry”, this paper by Hylleraas members  investigates the feasibility of using fully flexible explicitly correlated Gaussians for simulating laser-induced attosecond processes without the Born-Oppenheimer approximation.

For a full-size illustration, refer to the embedded figure in the article.

By Aleksander P. Wozniak, Ludwik Adamowicz, Thomas Bondo Pedersen, Simen Kvaal
Published May 15, 2024

The paper was published the 30 April 2024 by the Hylleraas members (authors): Simen Kvaal and Thomas Bondo Pedersen in collaboration with Aleksander Wozniak (University of Warsaw) and Ludwik Adamowicz (University of Arizona).

Read the article at: https://pubs.acs.org/doi/full/10.1021/acs.jpca.4c00364 

Summary/conclusion

Using two-dimensional model systems mimicking a hydrogenic electron and the coupled rotational and vibrational motion of a diatomic molecule, it is demonstrated that complicated ionization and bond-dissociation dynamics induced by strong laser pulses can be accurately described using relatively few Gaussian wave packets. This is achieved by fitting linear combinations of Gaussian wave packets to high-quality grid-based solutions of the time-dependent Schrödinger equation.

The results indicate that attosecond laser-driven electronic-nuclear quantum dynamics can be simulated by generalizing existing methodology from the time-independent to the time-dependent domain without assuming the Born-Oppenheimer approximation at any stage. 

Illustration.
Hydrogenic electron location probability density before, during, and after interaction with a strong laser pulse. Reproduced from J. Phys. Chem. A under CC-BY 4.0 license.
Tags: attosecond chemistry, Hylleraas, Gaussians, Born-Oppenheimer
Published May 15, 2024 2:07 PM - Last modified May 16, 2024 3:10 PM